4.结论

首次将Langmuir-Schaefer方法用于DEAs电极的制备。将多壁碳纳米管和聚（烷基噻吩）结合在一起，在空气-水界面形成稳定的单分子膜，然后使用Langmuir-Schaefer技术将其转移到PDMS膜上。单层电极由嵌入铂单层中的互连多壁碳纳米管网络组成，其中铂赋予机械性能，而多壁碳纳米管确保系统的导电性。复合单分子膜可拉伸，导电率高达100%(∼20 MΩ/0%应变时，∼5 GΩ/在100%应变下）。使用LS方法制作图案化超薄可拉伸电极，可以制作具有1.4μm厚PDMS介电膜的薄DEA。仅在100V下，该DEA达到4.0%线性应变。与DEAs通常需要的kV驱动电压相比，这种低工作电压为DEAs开辟了新的应用领域。我们在这里报告的LS电极是DEA在小于5V时产生全应变的关键构件：通过使用LS/LB技术制造弹性体和电极，将有可能制造多层DEA，其中所有层都是一个单分子厚度。这将是DEA技术的最终物理极限。

致谢

我们衷心感谢Jun Shintake博士、Matthias Imboden博士、Alexandre Poulin博士和Samuel Schlater先生的有益评论和讨论。这项工作是由欧盟的地平线2020研究和创新计划在玛丽SK·OOOWSKA居里补助金协议，第64 1822-MICACT通过瑞士国家教育、研究和创新秘书处，以及瑞士国家科学基金会授予第200020号165993。

附录A.补充数据

与本文相关的补充数据可在在线版本中找到，网址为https://doi.org/10.1016/j.snb.2018.01.145.

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